The presently disclosed embodiments relate in general to electrophotographic imaging members, such as layered photoreceptor structures, and processes for making and using the same. More particularly, the embodiments pertain to a photoreceptor undercoat layer that includes a metal oxide having a moisture content of less than 5 percent by weight of the total weight of the metal oxide, as well as, polyol and aminoplast resins, to improve image quality.