The present invention is directed toward cathodes and cathode materials comprising carbon nanotubes (CNTs) and particles. The present invention is also directed toward field emission devices comprising a cathode of the present invention, as well as methods for making these cathodes. In some embodiments, the cathode of the present invention is used in a field emission display. The invention also comprises a method of depositing a layer of CNTs and particles onto a substrate to form a cathode of the present invention, as well as a method of controlling the density of CNTs used in this mixed layer in an effort to optimize the field emission properties of the resulting layer for field emission display applications.